Wynne, K. (2005) A new ultrafast technique for measuring the terahertz dynamics of chiral molecules: the theory of optical heterodyne-detected Raman-induced Kerr optical activity. Journal of Chemical Physics, 122(24), p. 244503. (doi: 10.1063/1.1937390)
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Publisher's URL: http://dx.doi.org/10.1063/1.1937390
Abstract
Optical heterodyne-detected Raman-induced Kerroptical activity (OHD-RIKOA) is a nonresonant ultrafast chiroptical technique for measuring the terahertz-frequency Raman spectrum of chirally active modes in liquids, solutions, and glasses of chiral molecules. OHD-RIKOA has the potential to provide much more information on the structure of molecules and the symmetries of librational and vibrational modes than the well-known nonchirally sensitive technique optical heterodyne-detected Raman-induced Kerr-effect spectroscopy (OHD-RIKES). The theory of OHD-RIKOA is presented and possible practical ways of performing the experiments are analyzed.
Item Type: | Articles |
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Status: | Published |
Refereed: | Yes |
Glasgow Author(s) Enlighten ID: | Wynne, Professor Klaas |
Authors: | Wynne, K. |
College/School: | College of Science and Engineering > School of Chemistry |
Journal Name: | Journal of Chemical Physics |
Publisher: | American Institute of Physics |
ISSN: | 0021-9606 |
ISSN (Online): | 1089-7690 |
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