Generation of ultrafast terahertz radiation pulses on metallic nanostructured surfaces

Welsh, G.H. and Wynne, K. (2009) Generation of ultrafast terahertz radiation pulses on metallic nanostructured surfaces. Optics Express, 17(4), pp. 2470-2480. (doi: 10.1364/OE.17.002470)

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A resonant “incoherent” rectification process is presented relying on the excitation of surface plasmons on a nanostructured metal surface. Excitation of gold and silver films with 800-nm femtosecond laser pulses results in the emission of terahertz radiation with an angle-dependent efficiency and an approximately third-order power dependence. It is shown that the source of this terahertz pulse generation is the surface-plasmon-assisted multiphoton ionization and ponderomotive acceleration in the evanescent field of the surface plasmon. Simple models are used to understand the forces and dynamics near the surface.

Item Type:Articles
Glasgow Author(s) Enlighten ID:Wynne, Professor Klaas
Authors: Welsh, G.H., and Wynne, K.
College/School:College of Science and Engineering > School of Chemistry
Journal Name:Optics Express
Publisher:Optical Society of America
ISSN (Online):1094-4087

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Project CodeAward NoProject NamePrincipal InvestigatorFunder's NameFunder RefLead Dept
563561Terahertz spectroscopy of aqueous ionic solutions to understand the role of hydrogen-bond network breaking and strengthening in the HofmeisterKlaas WynneEngineering & Physical Sciences Research Council (EPSRC)EP/E046541/1CHEM - CHEMISTRY