Magnetically ordered and kagome quantum spin liquid states in the Zn-doped claringbullite series

Georgopoulou, M., Fak, B., Boldrin, D. , Stewart, J.R., Ritter, C., Suard, E., Ollivier, J. and Wills, A.S. (2023) Magnetically ordered and kagome quantum spin liquid states in the Zn-doped claringbullite series. Physical Review B, 107(2), 024416. (doi: 10.1103/PhysRevB.107.024416)

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Abstract

Neutron scattering measurements have been performed on deuterated powder samples of claringbullite and Zn-doped claringbullite [Zn x Cu 4 − x ( OD ) 6 FCl ]. At low temperatures, claringbullite Cu 4 ( OD ) 6 FCl forms a distorted pyrochlore lattice with long-range magnetic order and spin-wave-like magnetic excitations. Partial Zn doping leads to the nominal ZnCu 3 ( OD ) 6 FCl compound, a geometrically frustrated spin-1/2 kagome antiferromagnet that shows no transition to magnetic order down to 1.5 K. The magnetic excitations form a gapless continuum, a signature of fractional excitations in a quantum spin liquid.

Item Type:Articles
Status:Published
Refereed:Yes
Glasgow Author(s) Enlighten ID:Boldrin, Dr David
Authors: Georgopoulou, M., Fak, B., Boldrin, D., Stewart, J.R., Ritter, C., Suard, E., Ollivier, J., and Wills, A.S.
College/School:College of Science and Engineering > School of Physics and Astronomy
Journal Name:Physical Review B
Publisher:American Physical Society
ISSN:1098-0121
ISSN (Online):1550-235X
Published Online:17 January 2023

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