In-plane structural order of domain engineered La0.7Sr0.3MnO3thin films

Boschker, J.E., Monsen, Å.F., Nord, M., Mathieu, R., Grepstad, J.K., Holmestad, R., Wahlström, E. and Tybell, T. (2013) In-plane structural order of domain engineered La0.7Sr0.3MnO3thin films. Philosophical Magazine, 93(13), pp. 1549-1562. (doi: 10.1080/14786435.2012.747010)

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Abstract

We present a detailed structural study of tensile-strained La0.7Sr0.3MnO3 thin films. We use the substrate miscut to control the number of rhombohedral variants in the films and study the in-plane order and structural distortions. Using high-resolution X-ray diffraction, we demonstrate that step-edge induced lattice modulations occur in 4-variant films, whereas periodic twinning is the dominant in-plane order for 2-variant films. We show that the in-plane twinning angle is almost completely relaxed. However, the relaxation of shear strain by the out-of-plane twinning angle and the monoclinic distortion is only partial. Furthermore, the film thickness dependence of the domain width reveals that domain formation is a universal mechanism for shear strain relaxation. Finally, we show that the structural response to the transition from the paramagnetic to the ferromagnetic phase of La0.7Sr0.3MnO3 at 345 K is smaller in 4-variant films compared to 2-variant films.

Item Type:Articles
Status:Published
Refereed:Yes
Glasgow Author(s) Enlighten ID:Nord, Dr Magnus
Authors: Boschker, J.E., Monsen, Å.F., Nord, M., Mathieu, R., Grepstad, J.K., Holmestad, R., Wahlström, E., and Tybell, T.
College/School:College of Science and Engineering > School of Physics and Astronomy
Journal Name:Philosophical Magazine
Publisher:Taylor & Francis
ISSN:1478-6435
ISSN (Online):1478-6443
Published Online:29 November 2012

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