Sources of anthropogenic C-14 to the North Sea

Gulliver, P. , Cook, G.T., MacKenzie, A.B., Naysmith, P. and Anderson, R. (2004) Sources of anthropogenic C-14 to the North Sea. Radiocarbon, 46(2), pp. 869-875.

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Abstract

The Sellafield nuclear fuel reprocessing plant on the northwest coast of England is the largest source of anthropogenic radiocarbon to the UK coastal environment. In a mid-1990s study of C-14 distribution around the UK coast, the pattern of dilution with increasing distance from Sellafield appeared to be perturbed by anomalously high C-14 activities in marine biota in the coastal environment of northeast England. This present study was undertaken during 1998 and 1999 to determine whether this C-14 enhancement was due to Sellafield or the nuclear power plants on the east coast. Seawater, seaweed (Fucus sp.), and mussel (Mytilus edulis) samples that were collected from the vicinity of the Torness and Hartlepool advanced gas-cooled reactor (AGR) nuclear power stations were all enhanced above the contemporary regional background activity derived from natural production and atmospheric nuclear weapons testing. We used previously published dilution factors and transfer times for Tc-99 between Sellafield and various points on the UK coast to determine likely Sellafield- derived C-14 contributions to the activities at the nuclear power plant sites. The results suggest that the activities observed at Torness, which are only marginally enhanced above the natural background activity, are possibly due to discharges from Sellafield; however, the significant C-14 enhancements at Hartlepool are not Sellafield-derived. Furthermore, since both reactors have the same fundamental design, the low activities at the Torness AGR imply that the activities at Hartlepool are not from the AGR, suggesting that there is an input of C-14 to the marine environment in the vicinity of Hartlepool which is probably non-nuclear-power related. However, there is no other authorized site in the area that could account for the observed C-14 enrichments; therefore, further research is required to ascertain the source of this C-14.

Item Type:Articles
Status:Published
Refereed:Yes
Glasgow Author(s) Enlighten ID:Cook, Professor Gordon and Naysmith, Mr Philip and MacKenzie, Professor Angus and Anderson, Mr Robert and Gulliver, Dr Pauline
Authors: Gulliver, P., Cook, G.T., MacKenzie, A.B., Naysmith, P., and Anderson, R.
Subjects:Q Science > QD Chemistry
Q Science > QE Geology
College/School:College of Science and Engineering > Scottish Universities Environmental Research Centre
Journal Name:Radiocarbon
Publisher:University of Arizona
ISSN:0033-8222
Copyright Holders:© 2004 by the Arizona Board of Regents on behalf of the University of Arizona
First Published:First published in Radiocarbon 46(2):869-875
Publisher Policy:Reproduced with the permission of the Publisher.

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