Accelerated carbonation and performance of concrete made with steel slag as binding materials and aggregates

Mo, L., Zhang, F., Deng, M., Jin, F. , Al-Tabbaa, A. and Wang, A. (2017) Accelerated carbonation and performance of concrete made with steel slag as binding materials and aggregates. Cement and Concrete Composites, 83, pp. 138-145. (doi:10.1016/j.cemconcomp.2017.07.018)

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Abstract

Steel slag has been used as supplementary cementitious materials or aggregates in concrete. However, the substitution levels of steel slag for Portland cement or natural aggregates were limited due to its low hydraulic property or latent volume instability. In this study, 60% of steel slag powders containing high free-CaO content, 20% of Portland cement and up to 20% of reactive magnesia and lime were mixed to prepare the binding blends. The binding blends were then used to cast concrete, in which up to 100% of natural aggregates (limestone and river sands) were replaced with steel slag aggregates. The concrete was exposed to carbonation curing with a concentration of 99.9% CO2 and a pressure of 0.10 MPa for different durations (1d, 3d, and 14d). The carbonation front, carbonate products, compressive strength, microstructure, and volume stability of the concrete were investigated. Results show that the compressive strength of the steel slag concrete after CO2 curing was significantly increased. The compressive strengths of concrete subjected to CO2 curing for 14d were up to five-fold greater than that of the corresponding concrete under conventional moist curing for 28d. This is attributed to the formation of calcium carbonates, leading to a microstructure densification of the concrete. Replacement of limestone and sand aggregates with steel slag aggregates also increased the compressive strengths of the concrete subjected to CO2 curing. In addition, the concrete pre-exposed to CO2 curing produced less expansion than the concrete pre-exposed to moist curing during the subsequent accelerated curing in 60 °C water. This study provides a potential approach to prepare concrete with low-carbon emissions via the accelerated carbonation of steel slag.

Item Type:Articles
Additional Information:The authors are grateful to the financial supports from the open foundation of Anhui province key laboratory of advanced building materials of Anhui Jianzhu University (JZCL201601KF), National Natural Science Foundation of China (51461135003, 51502134, 51308004), EPSRC UK (EP/M003159/1), and the Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD).
Status:Published
Refereed:Yes
Glasgow Author(s) Enlighten ID:Jin, Dr Fei
Authors: Mo, L., Zhang, F., Deng, M., Jin, F., Al-Tabbaa, A., and Wang, A.
College/School:College of Science and Engineering > School of Engineering > Infrastructure and Environment
Journal Name:Cement and Concrete Composites
Publisher:Elsevier
ISSN:0958-9465
ISSN (Online):1873-393X
Published Online:23 July 2017
Copyright Holders:Copyright © 2017 The Authors
First Published:First published in Cement and Concrete Composites 83:138-145
Publisher Policy:Reproduced under a Creative Commons License

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